Solution structure of dynorphin A (1-17): a NMR study in a cryoprotective solvent mixture at 278 K

J Pept Sci. 1999 Jul;5(7):306-12. doi: 10.1002/(SICI)1099-1387(199907)5:7<306::AID-PSC199>3.0.CO;2-B.

Abstract

Dynorphin A, the endogenous agonist for the kappa opioid receptor, has been studied by NMR spectroscopy in methanol, acetonitrile, DMSO and in mixtures of hexafluoroacetone/water and DMSO/water. NMR data in the DMSO/water cryomixture at 278 K are consistent with a conformer in which the N-terminal part, like the corresponding message domain of enkephalins, is poorly ordered, whereas the C-terminal part is folded in a loop centred around Pro10. The folded structure of the C-terminal part (address moiety) may shed light on the role of the essential residues Arg7, Lys11 and Lys13.

MeSH terms

  • Amino Acid Sequence
  • Cold Temperature
  • Dynorphins / chemistry*
  • Humans
  • Magnetic Resonance Spectroscopy
  • Molecular Sequence Data
  • Nociceptin Receptor
  • Protein Conformation
  • Receptors, Opioid / chemistry
  • Receptors, Opioid, kappa / chemistry
  • Receptors, Opioid, mu / chemistry
  • Solutions
  • Solvents

Substances

  • Receptors, Opioid
  • Receptors, Opioid, kappa
  • Receptors, Opioid, mu
  • Solutions
  • Solvents
  • Dynorphins
  • Nociceptin Receptor
  • OPRL1 protein, human