Application of liquid chromatography-turbo ion spray tandem mass spectrometry for quantitative analysis of a potent motilin receptor agonist, EM574, and its metabolites in human plasma

J Chromatogr B Biomed Sci Appl. 1999 Oct 29;734(1):101-12. doi: 10.1016/s0378-4347(99)00335-7.

Abstract

A liquid chromatography-tandem mass spectrometry (LC-MS-MS) method for the simultaneous determination of a new potent motilin receptor agonist as erythromycin derivative, EM574 (erythromycin derivative), and its three metabolites, M-IV, M-V and M-VI, in human plasma was developed. The internal standards (I.S.s) used were deuterated EM574, M-IV and M-V. For the quantitation of M-VI, deuterated M-V was used. The analytes and I.S. were extracted from plasma samples with diethyl ether at neutral pH. A turbo ion spray interface was used as the ion source of LC-MS-MS, and the analysis was performed in the selected reaction monitoring mode. The lower quantitation limits for all the analytes were 0.05 ng/ml when 0.2 ml of plasma was used, and the standard curves were linear in the range 0.05 to 20 ng/ml. The method was precise; the intra- and inter-day precisions of the method were not more than 19.8% for all the analytes. The accuracy of the method was good with the deviations between added and calculated concentrations of each analyte being typically within +/- 11.2%.

MeSH terms

  • Chromatography, Liquid / methods*
  • Deuterium
  • Erythromycin / analogs & derivatives*
  • Erythromycin / blood
  • Erythromycin / chemistry
  • Erythromycin / metabolism
  • Gastrointestinal Agents / blood*
  • Gastrointestinal Agents / chemistry
  • Gastrointestinal Agents / metabolism
  • Humans
  • Hydrogen-Ion Concentration
  • Kinetics
  • Mass Spectrometry / methods*
  • Molecular Structure
  • Receptors, Gastrointestinal Hormone / agonists*
  • Receptors, Neuropeptide / agonists*
  • Sensitivity and Specificity

Substances

  • Gastrointestinal Agents
  • Receptors, Gastrointestinal Hormone
  • Receptors, Neuropeptide
  • motilin receptor
  • Idremcinal
  • Erythromycin
  • Deuterium