Species selectivity of a small molecule antagonist for the CCR1 chemokine receptor

Eur J Pharmacol. 2000 Feb 11;389(1):41-9. doi: 10.1016/s0014-2999(99)00863-8.

Abstract

The species specificity of a small molecule antagonist for the human CCR1 chemokine receptor, 2-2-diphenyl-5-(4-chlorophenyl)piperidin-1-yl)valeronitrile (CCR1 antagonist 1), has been examined using cloned CCR1 receptors from various species. The compound was able to bind to rabbit, marmoset, and human CCR1, and was able to block the functional activation of these receptors. However, it failed to significantly displace radiolabeled macrophage inflammatory protein-1alpha (MIP-1alpha) binding to mouse CCR1 at concentrations up to 10 microM. These data suggested that the antagonist binding site is well-conserved in rabbit, marmoset and human CCR1, but not in mouse CCR1. The functional selectivity and mechanism of action for CCR1 antagonist 1 were further characterized. CCR1 antagonist 1 blocked the increase in intracellular Ca(2+) stimulated by CCR1 agonists, but had no effect on N-formyl-Met-Leu-Phe (FMLP), monocyte chemotactic protein-1 (MCP-1) and stromal-derived factor 1alpha (SDF1alpha)-induced Ca(2+) mobilization, demonstrating functional selectivity for CCR1. Since CCR1 antagonist 1 is a functional antagonist of marmoset and rabbit CCR1 receptors, it should be possible to test its efficacy in animal models of disease.

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Binding Sites
  • Calcium / metabolism
  • Callithrix
  • Chemokine CCL3
  • Chemokine CCL4
  • Chemokine CCL5 / metabolism
  • Cloning, Molecular
  • DNA, Complementary / genetics
  • DNA, Complementary / metabolism
  • Humans
  • Macrophage Inflammatory Proteins / metabolism
  • Mice
  • Molecular Sequence Data
  • Nitriles / pharmacology*
  • Nitriles / toxicity
  • Piperazines / pharmacology*
  • Piperazines / toxicity
  • Piperidines / pharmacology
  • Piperidines / toxicity
  • Rabbits
  • Receptors, CCR1
  • Receptors, Chemokine / antagonists & inhibitors*
  • Receptors, Chemokine / genetics
  • Receptors, Chemokine / metabolism
  • Receptors, Chemokine / physiology
  • Species Specificity

Substances

  • 2,2-diphenyl-(5-(4-chlorophenyl)piperidin-1-yl)valeronitrile
  • CCR1 protein, human
  • Ccr1 protein, mouse
  • Chemokine CCL3
  • Chemokine CCL4
  • Chemokine CCL5
  • DNA, Complementary
  • Macrophage Inflammatory Proteins
  • Nitriles
  • Piperazines
  • Piperidines
  • Receptors, CCR1
  • Receptors, Chemokine
  • Calcium

Associated data

  • GENBANK/AF127527
  • GENBANK/AF127528