Imaging and mapping heparin-binding sites on single fibronectin molecules with atomic force microscopy

Biochemistry. 2000 Mar 28;39(12):3192-6. doi: 10.1021/bi991624o.

Abstract

Fibronectin is composed of multiple homologous repeats and contains many functional domains. Two major heparin-binding domains have previously been identified: the Hep I site near the amino terminus and the Hep II site near the carboxyl terminus. The Hep II site has been considered the high-affinity heparin-binding site based on studies of fibronectin fragments. However, few studies have been carried out on heparin binding by intact fibronectin. We imaged single fibronectin molecules as well as heparin-coated gold particles bound to whole dimeric plasma fibronectin molecules with tapping mode atomic force microscopy. We observed heparin-gold particles preferentially bound at two locations that correspond to the Hep I and Hep II sites. Quantitative analysis of images of individual fibronectin-heparin-gold complexes showed that almost twice as many heparin-gold particles bound to the N-terminal Hep I site compared to the Hep II site. In contrast to previous findings with fibronectin fragments, these results suggest that the Hep I site has a binding affinity higher than or comparable to the Hep II site in the intact fibronectin molecule.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Binding Sites
  • Cattle
  • Dimerization
  • Disulfides / chemistry
  • Fibronectins / chemistry*
  • Fibronectins / ultrastructure
  • Gold Colloid / chemistry
  • Heparin / chemistry*
  • Heparin / ultrastructure
  • Image Enhancement
  • Microscopy, Atomic Force
  • Peptide Fragments / chemistry
  • Peptide Fragments / ultrastructure
  • Peptide Mapping
  • Random Allocation
  • Serum Albumin / chemistry
  • Serum Albumin / ultrastructure

Substances

  • Disulfides
  • Fibronectins
  • Gold Colloid
  • Peptide Fragments
  • Serum Albumin
  • Heparin