Anti-tumour effects and pharmacokinetic profile of 17-(5'-isoxazolyl)androsta-4,16-dien-3-one (L-39) in mice: an inhibitor of androgen synthesis

Br J Cancer. 2000 Jul;83(1):74-82. doi: 10.1054/bjoc.2000.1136.

Abstract

17-(5'-Isoxazolyl)androsta-4,16-dien-3-one (L-39), a novel androstene derivative, was synthesized and evaluated in vitro and in vivo. L-39 showed potent and non-competitive inhibition of human testicular microsomal 17alpha-hydroxylase/C(17,20)-lyase with an IC50 value of 59 nM and Ki of 22 nM. L-39 also showed potent and competitive inhibition of 5alpha-reductase in human prostatic microsomes with IC50 and Ki values of 33 and 28 nM respectively. L-39 (5 microM) has also been shown to manifest anti-androgenic activity in cultures of human prostate cancer cell lines (LNCaP) by preventing the labelled synthetic androgen R1881 (5 nM) from binding to the androgen receptors. Androgen-dependent human prostate cancer xenografts (PC-82) were grown in nude mice and the effects of L-39 (50 mg kg(-1) day(-1)) on tumour growth and prostate-specific antigen (PSA) levels were determined after 28 days. L-39 significantly (P < 0.01) diminished tumour growth and wet weights to a similar extent as castration or flutamide treatment. L-39 also significantly (P < 0.01) reduced serum PSA levels by more than 80% in the mice bearing human prostate cancer xenografts. Pharmacokinetic studies were also conducted in male Balb/c mice. After subcutaneous administration of a single bolus dose, L-39 was rapidly absorbed into the systemic circulation. Peak plasma levels occurred at 0.75 h and then declined with a t(1/2) of 1.51 h. The bioavailability of L-39 after subcutaneous administration was 28.5%. These results demonstrate that L-39 is a potent inhibitor of androgen synthesis and is effective in reducing the growth of human prostate cancer xenografts in nude mice. Although improvements in the bioavailability are necessary, L-39 is a potential lead compound with this profile as an inhibitor of prostate cancer growth.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • 5-alpha Reductase Inhibitors*
  • Androgen Antagonists / pharmacokinetics
  • Androgen Antagonists / therapeutic use*
  • Androgens / biosynthesis*
  • Androstadienes / administration & dosage
  • Androstadienes / pharmacokinetics
  • Androstadienes / therapeutic use*
  • Animals
  • Antineoplastic Agents, Hormonal / pharmacokinetics
  • Antineoplastic Agents, Hormonal / therapeutic use*
  • Chromatography, High Pressure Liquid
  • Drug Screening Assays, Antitumor
  • Enzyme Inhibitors / pharmacokinetics
  • Enzyme Inhibitors / therapeutic use*
  • Humans
  • Injections, Intravenous
  • Injections, Subcutaneous
  • Male
  • Mice
  • Mice, Nude
  • Microsomes / enzymology
  • Neoplasm Proteins / antagonists & inhibitors
  • Neoplasm Transplantation
  • Prostate / enzymology
  • Prostatic Hyperplasia / enzymology
  • Prostatic Neoplasms / drug therapy
  • Prostatic Neoplasms / pathology
  • Steroid 17-alpha-Hydroxylase / antagonists & inhibitors*
  • Testis / enzymology
  • Transplantation, Heterologous
  • Tumor Cells, Cultured / drug effects
  • Tumor Cells, Cultured / metabolism

Substances

  • 17-(5'-isoxazolyl)androsta-4,16-dien-3-one
  • 5-alpha Reductase Inhibitors
  • Androgen Antagonists
  • Androgens
  • Androstadienes
  • Antineoplastic Agents, Hormonal
  • Enzyme Inhibitors
  • Neoplasm Proteins
  • Steroid 17-alpha-Hydroxylase