Synthesis of hybrid distamycin-cysteine labeled with 99mTc: a model for a novel class of cancer imaging agents

Bioorg Med Chem Lett. 2000 Jun 19;10(12):1397-400. doi: 10.1016/s0960-894x(00)00250-x.

Abstract

The synthesis of a hybrid constituted by distamycin A and cysteine labeled with the gamma-emitting radionuclide 99mTc to afford the conjugate complex 5 is reported. This new radiopharmaceutical is of potential interest as tumor imaging agent in diagnostic nuclear medicine. The preparation of the hybrid distamycin A-cysteine 4 has been achieved by coupling deformyldistamycin A and Boc-Dmt-OH. Compound 4 was then successfully labeled with 99mTc by reaction with the novel, high-electrophilic, metal-containing fragment [99mTc(N)(PP)]2+ (PP = diphosphine ligand) yielding the 1:1 complex 5.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cysteine / chemistry*
  • Distamycins / chemistry*
  • Humans
  • Neoplasms / diagnostic imaging*
  • Organotechnetium Compounds / chemistry*
  • Radionuclide Imaging
  • Radiopharmaceuticals / chemical synthesis*

Substances

  • Distamycins
  • Organotechnetium Compounds
  • Radiopharmaceuticals
  • stallimycin
  • Cysteine