Transannular Diels-Alder studies on the asymmetric total synthesis of chatancin: the pyranophane approach

Org Lett. 2000 Sep 7;2(18):2737-40. doi: 10.1021/ol006220z.

Abstract

[reaction: see text] A pathway is proposed for the biosynthesis of (+)-chatancin and (+)-sarcophytin linking these tetracycles to cembranoids by a pyranophane transannular Diels-Alder reaction. Preliminary synthetic results in this direction to reach macrocyclic dienedione 28 from farnesol are reported. Major synthetic steps include a Prins reaction, two enantioselective hydrogenations, and a macrocyclization via a beta-ketosulfoxide Michael-addition on an enone.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cnidaria / chemistry
  • Crystallography, X-Ray
  • Diterpenes / chemical synthesis*
  • Diterpenes / chemistry
  • Farnesol / chemistry
  • Platelet Activating Factor / antagonists & inhibitors
  • Stereoisomerism

Substances

  • Diterpenes
  • Platelet Activating Factor
  • chatancin
  • Farnesol