Selectively conjugated melittins for liposome time-resolved fluoroimmunoassay of theophylline in serum

Fresenius J Anal Chem. 2000 Apr;366(8):869-72. doi: 10.1007/s002160051587.

Abstract

Theophylline (Th) has been selectively conjugated to the four amino groups of melittin (Mel) by solid phase peptide synthesis. The cytolytic activity of the resultant Th-Mel compounds was tested on liposomes trapping the bovine serum albumin (BSA) conjugate with 4,7-bis(chlorosulfophenyl)-1,10-phenanthrol ine-2,9-dicarboxylic acid (BCPDA). The loss of lytic activity was the highest for Th-K7-Mel. Th-G1-Mel retains almost the same lytic activity as Mel. A homogeneous liposome time-resolved fluoroimmunoassay (LITRFIA) of Th in serum has been carried out with Th-G1-Mel between 5 ng and 10 microg.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Antibodies / immunology
  • Calibration
  • Dose-Response Relationship, Drug
  • Europium
  • Fluorescent Dyes / metabolism
  • Fluoroimmunoassay / methods*
  • Haptens / immunology
  • Humans
  • Liposomes / chemistry
  • Liposomes / metabolism*
  • Melitten / analogs & derivatives*
  • Melitten / metabolism
  • Melitten / pharmacology
  • Molecular Sequence Data
  • Permeability / drug effects
  • Phenanthrolines / metabolism
  • Sensitivity and Specificity
  • Serum Albumin / metabolism
  • Substrate Specificity
  • Theophylline / analogs & derivatives*
  • Theophylline / blood*
  • Theophylline / immunology

Substances

  • Antibodies
  • Fluorescent Dyes
  • Haptens
  • Liposomes
  • Phenanthrolines
  • Serum Albumin
  • 4,7-bis(chlorosulfophenyl)-1,10-phenanthroline-2,9-dicarboxylic acid
  • Melitten
  • Europium
  • Theophylline