Importance of vacutainer selection in forensic toxicological analysis of drugs of abuse

J Anal Toxicol. 2001 Jul-Aug;25(5):339-43. doi: 10.1093/jat/25.5.339.

Abstract

The enzymatic degradation of cocaine in blood samples, even during transport to a forensic laboratory, is a common problem in toxicological analysis. This can be avoided by the use of blood-sampling devices such as gray-top Vacutainers containing the cholinesterase inhibitor sodium fluoride. In the present study, which included 147 authentic cases, blood samples were collected into two different tubes, one containing fluoride/oxalate and one without stabilizing agents. In all cases, both samples were analyzed for drugs of abuse using Abbott FPIA immunoassays after precipitation and gas chromatography-mass spectrometry (GC-MS) for quantitative analysis. The cannabinoid immunoassay showed markedly lower values in the fluoride-containing samples; this was investigated further and could be explained by hemolysis of these samples. In addition, the concentrations of 11-nor-delta9-tetrahydrocannabinol-9-carboxylic acid (THCCOOH) were lower in these samples. A stability study with the THCCOOH acyl glucuronide showed that it is unstable in unpreserved serum, which could explain our observation. GC-MS quantitative data for amphetamine and derivatives, opiates, delta9-tetrahydrocannabinol, and 11-hydroxy-delta9-tetrahydrocannabinol were essentially identical; however, they also differed substantially for cocaine, cocaethylene, ecgonine methylester, and benzoylecgonine. Unexpectedly, the concentrations of benzoylecgonine in unpreserved serum were almost half as high as in the fluoride-containing samples.

MeSH terms

  • Automobile Driving / legislation & jurisprudence
  • Blood Specimen Collection / instrumentation*
  • Drug Stability
  • Forensic Medicine / instrumentation*
  • Forensic Medicine / methods
  • Gas Chromatography-Mass Spectrometry
  • Humans
  • Illicit Drugs / blood
  • Immunoassay
  • Substance Abuse Detection / instrumentation*
  • Substance Abuse Detection / legislation & jurisprudence
  • Substance Abuse Detection / methods

Substances

  • Illicit Drugs