A yeast sensor of ligand binding

Nat Biotechnol. 2001 Nov;19(11):1042-6. doi: 10.1038/nbt1101-1042.

Abstract

We describe a biosensor that reports the binding of small-molecule ligands to proteins as changes in growth of temperature-sensitive yeast. The yeast strains lack dihydrofolate reductase (DHFR) and are complemented by mouse DHFR containing a ligand-binding domain inserted in a flexible loop. Yeast strains expressing two ligand-binding domain fusions, FKBP12-DHFR and estrogen receptor-alpha (ERalpha)-DHFR, show increased growth in the presence of their corresponding ligands. We used this sensor to identify mutations in residues of ERalpha important for ligand binding, as well as mutations generally affecting protein activity or expression. We also tested the sensor against a chemical array to identify ligands that bind to FKBP12 or ERalpha. The ERalpha sensor was able to discriminate among estrogen analogs, showing different degrees of growth for the analogs that correlated with their relative binding affinities (RBAs). This growth assay provides a simple and inexpensive method to select novel ligands and ligand-binding domains.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Binding Sites
  • Biosensing Techniques / methods*
  • Cell Division
  • Estradiol Congeners / metabolism
  • Estrogen Receptor alpha
  • Gene Deletion
  • Kinetics
  • Ligands
  • Mice
  • Molecular Sequence Data
  • Mutation
  • Protein Structure, Tertiary
  • Receptors, Estrogen / chemistry
  • Receptors, Estrogen / genetics
  • Receptors, Estrogen / metabolism
  • Recombinant Fusion Proteins / metabolism
  • Saccharomyces cerevisiae / enzymology
  • Saccharomyces cerevisiae / genetics*
  • Saccharomyces cerevisiae / growth & development
  • Tacrolimus / metabolism
  • Tacrolimus Binding Protein 1A / genetics
  • Tacrolimus Binding Protein 1A / metabolism
  • Temperature
  • Tetrahydrofolate Dehydrogenase / genetics

Substances

  • Estradiol Congeners
  • Estrogen Receptor alpha
  • Ligands
  • Receptors, Estrogen
  • Recombinant Fusion Proteins
  • Tetrahydrofolate Dehydrogenase
  • Tacrolimus Binding Protein 1A
  • Tacrolimus