Contributions of folding cores to the thermostabilities of two ribonucleases H

Protein Sci. 2002 Feb;11(2):381-9. doi: 10.1110/ps.38602.

Abstract

To investigate the contribution of the folding cores to the thermodynamic stability of RNases H, we used rational design to create two chimeras composed of parts of a thermophilic and a mesophilic RNase H. Each chimera combines the folding core from one parent protein and the remaining parts of the other. Both chimeras form active, well-folded RNases H. Stability curves, based on CD-monitored chemical denaturations, show that the chimera with the thermophilic core is more stable, has a higher midpoint of thermal denaturation, and a lower change in heat capacity (DeltaCp) upon unfolding than the chimera with the mesophilic core. A possible explanation for the low DeltaCp of both the parent thermophilic RNase H and the chimera with the thermophilic core is the residual structure in the denatured state. On the basis of the studied parameters, the chimera with the thermophilic core resembles a true thermophilic protein. Our results suggest that the folding core plays an essential role in conferring thermodynamic parameters to RNases H.

Publication types

  • Comparative Study
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Chimera
  • Circular Dichroism
  • Enzyme Stability
  • Escherichia coli / enzymology
  • Hot Temperature
  • Models, Molecular
  • Molecular Sequence Data
  • Plasmids
  • Polymerase Chain Reaction
  • Protein Denaturation
  • Protein Folding
  • Ribonuclease H / chemistry*
  • Sequence Homology, Amino Acid
  • Thermodynamics
  • Thermus thermophilus / enzymology*
  • X-Ray Diffraction

Substances

  • Ribonuclease H

Associated data

  • PDB/1F121
  • PDB/1JL2