Enantioselective synthesis of marine indole alkaloid hamacanthin B

J Org Chem. 2002 Feb 22;67(4):1396-8. doi: 10.1021/jo0108109.

Abstract

An enantioselective total synthesis of hamacanthin B (1) is described. This synthesis is based on the asymmetric synthesis of (S)-2-azido-(indol-3-yl)ethylamine 7, which is coupled with the 3-indolyl-alpha-oxoacetyl chloride 8 and subsequently used in a successful intramolecular Staudinger-aza Wittig cyclization to form the central dihydropyrazinone ring. The stereochemistry of naturally isolated hamacanthin B is revealed as the (S)-configuration.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkaloids / chemical synthesis*
  • Alkaloids / chemistry
  • Animals
  • Catalysis
  • Indole Alkaloids
  • Indoles / chemical synthesis*
  • Indoles / chemistry
  • Magnetic Resonance Spectroscopy
  • Molecular Structure
  • Porifera / chemistry*
  • Pyrazines / chemical synthesis*
  • Pyrazines / chemistry
  • Stereoisomerism

Substances

  • Alkaloids
  • Indole Alkaloids
  • Indoles
  • Pyrazines
  • hamacanthine B