Functional proteomics using microchannel plate detectors

Proteomics. 2002 Mar;2(3):256-61. doi: 10.1002/1615-9861(200203)2:3<256::aid-prot256>3.0.co;2-k.

Abstract

We describe the development of a novel detection system used for the functional imaging of proteins separated on electrophoretic gels. A microchannel plate detector is used here for real-time imaging of low levels of tritiated protein separated by two-dimensional (2-D) electrophoresis. The system employs radioisotope-free, low noise microchannel plates originally developed for photon counting in X-ray astronomy. Using the detector configuration described here, proteins were resolved on mini gels by either one or two-dimensional electrophoresis, transferred onto polyvinylidene difluoride membranes and directly imaged. Tritiated diisopropylfluorophosphate (DFP) was used as a selective label for the serine hydrolase class of enzymes and their distribution in the central nervous system was examined. This survey revealed approximately 24 protein spots by 2-D electrophoresis. We also investigated the relative sensitivity of these proteins towards DFP and found the peptidase, acylpeptide hydrolase to be the most sensitive brain protein towards this reagent. Using a number of different tritiated standards, it was found that the system can image as little as 0.1 Bq/mm(2) of tritium corresponding to 320 attomol of DFP labelled protein/mm(2). Moreover, the system has a wide dynamic range (>10(6)) allowing samples of high and low activity to be quantified on the same gel.

MeSH terms

  • Animals
  • Brain Chemistry
  • Electrophoresis, Gel, Two-Dimensional / instrumentation*
  • Electrophoresis, Gel, Two-Dimensional / methods*
  • Image Processing, Computer-Assisted / methods*
  • Male
  • Proteome*
  • Rats
  • Rats, Inbred F344
  • Statistics as Topic
  • Tissue Extracts / chemistry

Substances

  • Proteome
  • Tissue Extracts