The putative effector-binding site of Leishmania mexicana pyruvate kinase studied by site-directed mutagenesis

FEBS Lett. 2002 Mar 13;514(2-3):255-9. doi: 10.1016/s0014-5793(02)02374-8.

Abstract

The activity of pyruvate kinase of Leishmania mexicana is allosterically regulated by fructose 2,6-bisphosphate (F-2,6-P(2)), contrary to the pyruvate kinases from other eukaryotes that are usually stimulated by fructose 1,6-bisphosphate (F-1,6-P(2)). Based on the comparison of the three-dimensional structure of Saccharomyces cerevisiae pyruvate kinase crystallized with F-1,6-P(2) present at the effector site (R-state) and the L. mexicana enzyme crystallized in the T-state, two residues (Lys453 and His480) were proposed to bind the 2-phospho group of the effector. This hypothesis was tested by site-directed mutagenesis. The allosteric activation by F-2,6-P(2) appeared to be entirely abrogated in the mutated enzymes confirming our predictions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Allosteric Regulation / drug effects
  • Allosteric Regulation / physiology
  • Amino Acid Substitution / physiology
  • Animals
  • Binding Sites / physiology
  • Enzyme Activation / drug effects
  • Enzyme Activation / physiology
  • Escherichia coli / genetics
  • Fructosediphosphates / pharmacology
  • Kinetics
  • Leishmania mexicana / enzymology*
  • Models, Molecular
  • Mutagenesis, Site-Directed
  • Protozoan Proteins / chemistry
  • Protozoan Proteins / genetics
  • Pyruvate Kinase / chemistry*
  • Pyruvate Kinase / genetics*
  • Saccharomyces cerevisiae / enzymology
  • Structure-Activity Relationship

Substances

  • Fructosediphosphates
  • Protozoan Proteins
  • fructose 2,6-diphosphate
  • Pyruvate Kinase