Anti-rheumatoid arthritis effect of the Kochia scoparia fruits and activity comparison of momordin lc, its prosapogenin and sapogenin

Arch Pharm Res. 2002 Jun;25(3):336-42. doi: 10.1007/BF02976636.

Abstract

MeOH extract of Kochia scoparia was fractionated into CHCl3-, EtOAc- and BuOH extracts and the last fraction were hydrolyzed by 3%-NaOH (MeOH-H2O) to compare the bioactivities on antinociceptive and anti-inflammatory effects. Silica gel column chromatography of BuOH fraction afforded a large amount of 3-O-beta-D-xylopyranosyl (1-->3)-beta-D-glucuronopyranosyl oleanolic acid (momordin lc, 4) and that of acid hydrolysate of BuOH fraction gave 3-O-beta-D-glucuronopyranosyl oleanolic acid (momordin lb, 3), its 6'-O-methyl ester (2) and oleanolic acid (1). Silica gel column chromatography of alkaline hydrolysate afforded a large amount of 4. MeOH extract and both EtOAc- and BuOH fractions were active in the rheumatoidal rat induced Freund's complete adjuvant reagent (FCA) whereas CHCl3 fraction was inactive. Compound 1 and 4 showed significant activities in the same assay but oleanolic acid 3-O-glucuronopyranoside (3) showed no activity. These fashions were also observed in carrageenan-induced edema of the rat and in the antinociceptive activity tests undertaken in hot plate- and writhing methods. These results suggest that momordin lc and its aglycone, oleanolic acid, could be active principles for rheumatoid arthritis.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetic Acid
  • Animals
  • Arthritis, Experimental / drug therapy*
  • Carrageenan
  • Chenopodiaceae / chemistry*
  • Edema / chemically induced
  • Edema / prevention & control
  • Fruit / chemistry*
  • Hydrolysis
  • Male
  • Mice
  • Mice, Inbred ICR
  • Oleanolic Acid / analogs & derivatives
  • Oleanolic Acid / isolation & purification
  • Oleanolic Acid / pharmacology
  • Oleanolic Acid / therapeutic use*
  • Pain Measurement / drug effects
  • Plant Extracts / chemistry
  • Rats
  • Rats, Sprague-Dawley
  • Sapogenins / therapeutic use
  • Structure-Activity Relationship

Substances

  • Plant Extracts
  • Sapogenins
  • momordin I (Oleanolic Acid)
  • Oleanolic Acid
  • Carrageenan
  • Acetic Acid