Insights into trehalose synthesis provided by the structure of the retaining glucosyltransferase OtsA

Chem Biol. 2002 Dec;9(12):1337-46. doi: 10.1016/s1074-5521(02)00292-2.

Abstract

Trehalose is a nonreducing disaccharide that plays a major role in many organisms, most notably in survival and stress responses. In Mycobacterium tuberculosis, it plays a central role as the carbohydrate core of numerous immunogenic glycolipids including "cord factor" (trehalose 6,6'-dimycolate). The classical pathway for trehalose synthesis involves the condensation of UDP-glucose and glucose-6-phosphate to afford trehalose-6-phosphate, catalyzed by the retaining glycosyltransferase OtsA. The configurations of two anomeric positions are set simultaneously, resulting in the formation of a double glycoside. The three-dimensional structure of the Escherichia coli OtsA, in complex with both UDP and glucose-6-phosphate, reveals the active site at the interface of two beta/alpha/beta domains. The overall structure and the intimate details of the catalytic machinery reveal a striking similarity to glycogen phosphorylase, indicating a strong evolutionary link and suggesting a common catalytic mechanism.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Binding Sites
  • Catalytic Domain
  • Glucosyltransferases / chemistry*
  • Glucosyltransferases / metabolism
  • Models, Molecular
  • Phosphorylases / chemistry
  • Protein Conformation
  • Sequence Alignment
  • Structural Homology, Protein
  • Trehalose / biosynthesis*

Substances

  • Trehalose
  • Glucosyltransferases
  • Phosphorylases
  • trehalose-6-phosphate synthase