Effects of endogenous agonists, glycine and D-serine, on in vivo specific binding of [11C]L-703,717, a PET radioligand for the glycine-binding site of NMDA receptors

Synapse. 2003 Nov;50(2):130-6. doi: 10.1002/syn.10254.

Abstract

A positron-emitter (carbon-11) labeled antagonist for the glycine-binding site of NMDA receptors, [(11)C]L-703,717, has a unique in vivo binding characteristic, in which it preferentially binds to cerebellar-specific NMDA receptors consisting of a GluRepsilon3 subunit and eventually accumulates in rodent cerebellum under in vivo conditions, but not under in vitro conditions. In order to understand the in vivo-specific site and subunit localization of this radioligand, we examined the effect of the endogenous glycine site agonists, glycine and D-serine, on in vivo [(11)C]L-703,717 binding. An increase in extracellular glycine concentration by treatment with a glycine transporter 1 (GlyT1)-selective inhibitor, NFPS ethyl ester, significantly decreased the cerebellar localization of [(11)C]L-703,717 in rats. D-serine is known to be concentrated in mammalian forebrain regions. The lack of D-serine detection in the cerebellum may be due to the fact that it has the highest enzymatic activity of D-amino acid oxidase (DAO). It was found that the cerebellar localization of [(11)C]L-703,717 is greatly diminished in mutant mice lacking DAO, in which D-serine content in the cerebellum is drastically increased from a nondetectable level in normal mice. These studies indicate that [(11)C]L-703,717 is susceptible to inhibition by glycine site agonists in its in vivo binding, and suggest that regional differences in inhibitions by endogenous agonists may be a crucial factor in the site- and subunit-specific binding of this glycine-site antagonist.

MeSH terms

  • Amino Acid Transport Systems, Neutral / antagonists & inhibitors
  • Amino Acid Transport Systems, Neutral / metabolism
  • Animals
  • Binding Sites / drug effects
  • Binding Sites / physiology
  • Binding, Competitive / drug effects
  • Binding, Competitive / genetics
  • Carbon Radioisotopes
  • Cerebellum / diagnostic imaging
  • Cerebellum / drug effects
  • Cerebellum / metabolism
  • D-Amino-Acid Oxidase / deficiency
  • D-Amino-Acid Oxidase / genetics
  • Extracellular Fluid / drug effects
  • Extracellular Fluid / metabolism
  • Glycine / metabolism
  • Glycine / pharmacology*
  • Glycine Plasma Membrane Transport Proteins
  • Hydroxyquinolines / pharmacokinetics*
  • Ligands
  • Male
  • Mice
  • Mice, Knockout
  • Neurons / diagnostic imaging
  • Neurons / drug effects*
  • Neurons / metabolism
  • Quinolones / pharmacokinetics*
  • Radioligand Assay
  • Radionuclide Imaging
  • Rats
  • Rats, Sprague-Dawley
  • Receptors, N-Methyl-D-Aspartate / agonists*
  • Receptors, N-Methyl-D-Aspartate / metabolism
  • Sarcosine / analogs & derivatives*
  • Sarcosine / pharmacology
  • Serine / metabolism
  • Serine / pharmacology*
  • Stereoisomerism
  • Synaptic Transmission / drug effects*
  • Synaptic Transmission / physiology
  • Up-Regulation / drug effects
  • Up-Regulation / physiology

Substances

  • Amino Acid Transport Systems, Neutral
  • Carbon Radioisotopes
  • Glycine Plasma Membrane Transport Proteins
  • Hydroxyquinolines
  • L 703717
  • Ligands
  • N-(3-(4'-fluorophenyl)-3-(4'-phenylphenoxy)-3-(4'-phenylphenoxy)propyl)sarcosine
  • NR2C NMDA receptor
  • Quinolones
  • Receptors, N-Methyl-D-Aspartate
  • Slc6a9 protein, mouse
  • Slc6a9 protein, rat
  • Serine
  • D-Amino-Acid Oxidase
  • Glycine
  • Sarcosine