Single-molecule kinetics of lambda exonuclease reveal base dependence and dynamic disorder

Science. 2003 Aug 29;301(5637):1235-8. doi: 10.1126/science.1084387.

Abstract

We used a multiplexed approach based on flow-stretched DNA to monitor the enzymatic digestion of lambda-phage DNA by individual bacteriophage lambda exonuclease molecules. Statistical analyses of multiple single-molecule trajectories observed simultaneously reveal that the catalytic rate is dependent on the local base content of the substrate DNA. By relating single-molecule kinetics to the free energies of hydrogen bonding and base stacking, we establish that the melting of a base from the DNA is the rate-limiting step in the catalytic cycle. The catalytic rate also exhibits large fluctuations independent of the sequence, which we attribute to conformational changes of the enzyme-DNA complex.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Bacteriophage lambda / enzymology*
  • Base Composition
  • Base Sequence
  • Binding Sites
  • Catalysis
  • DNA, Single-Stranded / chemistry
  • DNA, Single-Stranded / metabolism*
  • DNA, Viral / chemistry
  • DNA, Viral / metabolism*
  • Exodeoxyribonucleases / chemistry
  • Exodeoxyribonucleases / metabolism*
  • Hydrogen Bonding
  • Hydrolysis
  • Kinetics
  • Nucleic Acid Conformation
  • Protein Conformation
  • Thermodynamics
  • Viral Proteins

Substances

  • DNA, Single-Stranded
  • DNA, Viral
  • Viral Proteins
  • Exodeoxyribonucleases
  • exo protein, Bacteriophage lambda