Metabolic stability and tumor inhibition of bombesin/GRP receptor antagonists

Peptides. 1992 Mar-Apr;13(2):401-7. doi: 10.1016/0196-9781(92)90128-p.

Abstract

Small cell lung cancers (SCLC) synthesize and secrete bombesin/gastrin releasing peptide (BN/GRP). The autocrine growth cycle of BN/GRP in SCLC can be disrupted by BN/GRP receptor antagonists such as [Psi13,14]BN. Here several BN analogues were solid-phase synthesized and incubated with intact SCLC cells at 37 degrees C in RPMI medium in a time-course fashion (0-1080 minutes) to determine enzymatic stability. The proteolytic stability of the compounds was determined by subsequent HPLC analysis. The metabolic half-life ranged from 154 minutes to 1388 minutes for the six analogues studied. [Psi13,14]BN was found to be very stable to metabolic enzymes (T1/2 = 646 mm) and also inhibited SCLC xenograft formation in vivo in a dose-dependent manner. When [Psi13,14]BN was incubated with NCI-H345 cells, it inhibited 125I-GRP binding with an IC50 value of 30 nM. These data suggest that BN/GRP receptor antagonists such as [Psi13,14]BN may be useful for the treatment of SCLC.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Antineoplastic Agents / metabolism
  • Antineoplastic Agents / pharmacology*
  • Bombesin / metabolism*
  • Bombesin / pharmacology
  • Carcinoma, Small Cell / drug therapy*
  • Carcinoma, Small Cell / metabolism
  • Cell Division / drug effects
  • Cell Line
  • Female
  • Gastrin-Releasing Peptide
  • Half-Life
  • Kinetics
  • Mice
  • Mice, Inbred BALB C
  • Mice, Nude
  • Molecular Sequence Data
  • Peptides / metabolism*
  • Peptides / pharmacology
  • Receptors, Bombesin
  • Receptors, Neurotransmitter / analysis
  • Receptors, Neurotransmitter / antagonists & inhibitors*
  • Second Messenger Systems / drug effects
  • Tumor Cells, Cultured

Substances

  • Antineoplastic Agents
  • Peptides
  • Receptors, Bombesin
  • Receptors, Neurotransmitter
  • Gastrin-Releasing Peptide
  • Bombesin