Photoaffinity labeling of the phylloquinone-binding polypeptides by 2-azidoanthraquinone in photosystem I particles

FEBS Lett. 1992 Nov 2;312(1):27-30. doi: 10.1016/0014-5793(92)81403-9.

Abstract

A photoaffinity label, 2-azido-9,10-anthraquinone, binds at the quinone-binding (Q phi) site with high affinity and can substitute for the secondary acceptor, phylloquinone, in photosystem I reaction center of spinach. Phylloquinone-depleted photosystem I particles reconstituted with azido[3H]anthraquinone were illuminated with UV light and analyzed by sodium dodecylsulfate-polyacrylamide gel electrophoresis. The large core polypeptides (psaA and/or psaB) were selectively labeled. The labeling was competitively inhibited in the presence of anthraquinone. These results indicate that the Q phi site is located on psaA or psaB polypeptides.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Affinity Labels / metabolism*
  • Anthraquinones / metabolism*
  • Azides / metabolism*
  • Binding Sites
  • Chloroplasts / metabolism
  • Electrophoresis, Polyacrylamide Gel
  • Kinetics
  • Molecular Weight
  • Peptide Fragments / isolation & purification
  • Photosynthetic Reaction Center Complex Proteins / isolation & purification
  • Photosynthetic Reaction Center Complex Proteins / metabolism*
  • Photosystem I Protein Complex
  • Plants / metabolism*
  • Spectrophotometry
  • Vitamin K 1 / metabolism*

Substances

  • Affinity Labels
  • Anthraquinones
  • Azides
  • Peptide Fragments
  • Photosynthetic Reaction Center Complex Proteins
  • Photosystem I Protein Complex
  • 2-azidoanthraquinone
  • Vitamin K 1