Development of a fluorescence polarization assay to screen for inhibitors of the FtsZ/ZipA interaction

Anal Biochem. 2003 Dec 15;323(2):224-33. doi: 10.1016/j.ab.2003.08.033.

Abstract

A fluorescence polarization competition assay has been developed to screen for inhibitors of the Escherichia coli FtsZ/ZipA protein-protein interaction. A previously published X-ray costructure demonstrated that a 17-amino-acid peptide, corresponding to FtsZ C-terminal residues 367-383 (FtsZ(367-383)), interacts with the C-terminal FtsZ binding domain of ZipA (ZipA(185-328)). Phage display was employed to identify a unique but related peptide which when further modified and labeled was shown to have a higher affinity to ZipA(185-328) than the FtsZ(367-383) peptide and binds to the same site. This peptide had a six fold increase in fluorescence polarization upon binding to ZipA(185-328) compared to a two fold increase for the FtsZ(367-383) fluorophore. As a result, assay parameters using the phage display peptide were further optimized and adapted for the high-throughput screen. A high-throughput screen of 250,000 compounds identified 29 hits with inhibition equal to or greater than 30% at 50 microg/ml. An X-ray costructure of a promising small molecule in this library complexed with ZipA(185-328) (KI=12 microM) revealed that the compound binds to the same hydrophobic pocket as the FtsZ(367-383) peptide.

Publication types

  • Evaluation Study

MeSH terms

  • Amino Acid Sequence
  • Bacterial Proteins / antagonists & inhibitors*
  • Bacterial Proteins / metabolism
  • Binding, Competitive
  • Carrier Proteins / antagonists & inhibitors*
  • Carrier Proteins / metabolism
  • Cell Cycle Proteins / antagonists & inhibitors*
  • Cell Cycle Proteins / metabolism
  • Cytoskeletal Proteins / antagonists & inhibitors*
  • Cytoskeletal Proteins / metabolism
  • Dimethyl Sulfoxide / pharmacology
  • Escherichia coli / drug effects
  • Escherichia coli / metabolism
  • Escherichia coli Proteins / antagonists & inhibitors*
  • Escherichia coli Proteins / metabolism
  • Fluorescence Polarization / methods*
  • Models, Biological
  • Models, Molecular
  • Molecular Sequence Data
  • Peptide Fragments / metabolism
  • Protein Binding / drug effects
  • Protein Binding / physiology
  • Pyrimidines / pharmacology
  • Structure-Activity Relationship
  • Surface-Active Agents / pharmacology

Substances

  • Bacterial Proteins
  • Carrier Proteins
  • Cell Cycle Proteins
  • Cytoskeletal Proteins
  • Escherichia coli Proteins
  • FtsZ protein, Bacteria
  • Peptide Fragments
  • Pyrimidines
  • Surface-Active Agents
  • ZipA protein, E coli
  • Dimethyl Sulfoxide