Probing the molecular environment using spin-resolved photoelectron spectroscopy

Phys Rev Lett. 2004 Jan 9;92(1):013001. doi: 10.1103/PhysRevLett.92.013001. Epub 2004 Jan 8.

Abstract

Angle- and spin-resolved photoelectron spectroscopy with linearly and circularly polarized synchrotron radiation were used to study the electronic structure of model triatomic molecules, hydrogen sulfide, and carbonyl sulfide. The spin-polarization measurements of the molecular field split components of the S 2p photolines revealed a strong effect of the different molecular environments. The validity of simple atomic models to explain the results is discussed.