Rare and unexpected coordination to copper(II) by a tertiary amide in a macrocyclic ligand

Dalton Trans. 2004 Oct 21:(20):3163-5. doi: 10.1039/b410525g. Epub 2004 Sep 22.

Abstract

Incorporation of a tertiary amide donor within the framework of a C(2)-symmetric analogue of 1,4,7-triazacyclononane derived from L-valine results in the isolation of a very rare example of a classical Werner copper(II) complex in which tertiary amide coordination occurs; despite the monomeric nature of the complex in the solid state, frozen solution EPR studies reveal the presence of a triplet ground state consistent with a dimeric species.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amides / chemistry*
  • Copper / chemistry*
  • Crystallography, X-Ray
  • Electron Spin Resonance Spectroscopy
  • Macrocyclic Compounds / chemistry*
  • Organometallic Compounds / chemistry
  • Valine / chemistry

Substances

  • Amides
  • Macrocyclic Compounds
  • Organometallic Compounds
  • Copper
  • Valine