Room-temperature amplified spontaneous emission at 1300 nm in solution-processed PbS quantum-dot films

Opt Lett. 2005 Jan 15;30(2):171-3. doi: 10.1364/ol.30.000171.

Abstract

We report room-temperature amplified spontaneous emission and spectral narrowing at infrared wavelengths in solution-processed films made up of PbS quantum-dot nanocrystals. The results are relevant to optical amplification and lasing integrated upon a variety of substrates. The active optical medium operates at room temperature without any additional matrix material, providing an optical gain of 260 cm(-1) and a pump threshold of 1 mJ/cm(-2). Nanocrystals synthesized in an aqueous solution and stabilized by use of short ligands result in high quantum-dot volume fractions in solid films and in a redshift emission relative to absorption.

Publication types

  • Evaluation Study

MeSH terms

  • Complex Mixtures / analysis*
  • Complex Mixtures / chemistry*
  • Lead / chemistry*
  • Lead / radiation effects*
  • Membranes, Artificial*
  • Quantum Dots*
  • Spectrophotometry, Infrared / methods*
  • Sulfides / chemistry*
  • Sulfides / radiation effects*
  • Temperature

Substances

  • Complex Mixtures
  • Membranes, Artificial
  • Sulfides
  • lead sulfide
  • Lead