Hydroquinone modulates reactivity of peroxynitrite and nitric oxide production

J Pharm Pharmacol. 2005 Apr;57(4):475-81. doi: 10.1211/0022357055731.

Abstract

Peroxynitrite (ONOO(-)), a potent cytotoxic oxidant formed by the reaction of nitric oxide ((.-)NO) and superoxide radical ((.-)O(2)(-)), may be rapidly lethal in a cellular milieu due to oxidization and nitration processes. In the present study, hydroquinone displayed strong ONOO(-) scavenging activity and inhibitory effect on NO production in murine macrophage RAW264.7 cells. Hydroquinone strongly scavenged ONOO(-)induced dihydrorhodamine 123 oxidation in a dose-dependent manner compared with other reactive species such as (.-)O(2)(-) and (.-)NO. Hydroquinone also decreased levels of ONOO(-) induced nitrotyrosine of glutathione reductase and consequently prevented the enzyme from ONOO(-) induced damage. Furthermore, hydroquinone suppressed NO production, a cellular pathway for ONOO(-) formation, in lipopolysaccharide-activated RAW264.7 cells via inhibition of inducible NO synthase expression. The inhibitory effect by hydroquinone seems to be mediated by interruption of lipopolysaccharide-induced signalling such as activation of nuclear factor-kappaB and extracellular signalrelated kinases 1 and 2. The results suggest that hydroquinone may potently modulate reactivity of ONOO(-) and may therefore be a useful agent against ONOO(-) mediated diseases.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antioxidants / pharmacology*
  • Cell Line
  • Cell Survival / drug effects
  • Fluorescent Dyes
  • Free Radical Scavengers / pharmacology
  • Hydroquinones / pharmacology*
  • Lipopolysaccharides
  • Mitogen-Activated Protein Kinase 1 / metabolism
  • Mitogen-Activated Protein Kinase 3 / metabolism
  • NF-kappa B / metabolism
  • Nitrates / metabolism
  • Nitric Oxide / metabolism*
  • Nitric Oxide Synthase / antagonists & inhibitors
  • Nitrites / metabolism
  • Peroxynitrous Acid / metabolism*
  • Quercetin / pharmacology
  • Rhodamines
  • Superoxides / metabolism

Substances

  • Antioxidants
  • Fluorescent Dyes
  • Free Radical Scavengers
  • Hydroquinones
  • Lipopolysaccharides
  • NF-kappa B
  • Nitrates
  • Nitrites
  • Rhodamines
  • dihydrorhodamine 123
  • Superoxides
  • Peroxynitrous Acid
  • Nitric Oxide
  • Quercetin
  • Nitric Oxide Synthase
  • Mitogen-Activated Protein Kinase 1
  • Mitogen-Activated Protein Kinase 3
  • hydroquinone