Proton and phosphorus-31 nuclear magnetic resonance spectroscopy of human bile in hepatopancreaticobiliary cancer

Eur J Gastroenterol Hepatol. 2005 Jul;17(7):733-8. doi: 10.1097/00042737-200507000-00007.

Abstract

Objective: Hepatopancreaticobiliary cancers can be difficult to diagnose. Nuclear magnetic resonance (NMR) spectroscopy provides non-invasive information on phospholipid metabolism, and previous studies of liver tissue have highlighted changes in phospholipids in malignancy. We hypothesised that in-vitro NMR spectroscopy of human bile may provide independent diagnostic indices in cancer management through an assessment of the phospholipid content.

Design and methods: Bile samples from 24 patients were collected at endoscopic retrograde cholangiopancreatography and from one subject at cholecystectomy. Thirteen patients had cancer: pancreatic carcinoma (eight), cholangiocarcinoma (three) and metastatic liver disease (two). The remaining 12 patients had non-malignant pathology. In-vitro proton (H) and phosphorus-31 (P) NMR spectra were obtained from all samples using an 11.7 Tesla NMR spectroscopy system.

Results: Complementary information was obtained from the H and P NMR spectra. Signals were assigned to phosphatidylcholine in both H and P NMR spectra. Phosphatidylcholine levels were significantly reduced in the bile from cancer patients when compared with bile from non-cancer patients (P=0.007).

Conclusion: These preliminary studies suggest that H and P NMR spectroscopy of bile may be used to detect differences in phospholipid content between cancer and non-cancer patients. This may have implications for the development of novel diagnostic strategies in hepatopancreaticobiliary cancers. Further larger-scale studies are warranted.

MeSH terms

  • Adult
  • Aged
  • Aged, 80 and over
  • Bile / chemistry*
  • Bile Duct Neoplasms / chemistry*
  • Bile Duct Neoplasms / diagnostic imaging
  • Bile Duct Neoplasms / surgery
  • Bile Ducts, Intrahepatic / chemistry
  • Bile Ducts, Intrahepatic / diagnostic imaging
  • Bile Ducts, Intrahepatic / surgery
  • Cholangiocarcinoma / chemistry
  • Cholangiocarcinoma / diagnostic imaging
  • Cholangiocarcinoma / surgery
  • Cholangiopancreatography, Endoscopic Retrograde / methods
  • Cholecystectomy, Laparoscopic / methods
  • Female
  • Humans
  • Liver Neoplasms / chemistry*
  • Liver Neoplasms / diagnostic imaging
  • Liver Neoplasms / surgery
  • Magnetic Resonance Spectroscopy / methods*
  • Male
  • Middle Aged
  • Pancreatic Neoplasms / chemistry*
  • Pancreatic Neoplasms / diagnostic imaging
  • Pancreatic Neoplasms / surgery
  • Phospholipids / analysis
  • Phosphorus Isotopes
  • Pilot Projects
  • Protons

Substances

  • Phospholipids
  • Phosphorus Isotopes
  • Protons