The farnesyltransferase inhibitor L744832 potentiates UCN-01-induced apoptosis in human multiple myeloma cells

Clin Cancer Res. 2005 Jun 15;11(12):4589-600. doi: 10.1158/1078-0432.CCR-04-2346.

Abstract

Purpose: The purpose of this study was to characterize interactions between the farnesyltransferase inhibitor L744832 and the checkpoint abrogator UCN-01 in drug-sensitive and drug-resistant human myeloma cell lines and primary CD138+ multiple myeloma cells.

Experimental design: Wild-type and drug-resistant myeloma cell lines were exposed to UCN-01 +/- L744832 for 24 hours, after which mitochondrial injury, caspase activation, apoptosis, and various perturbations in signaling and survival pathways were monitored.

Results: Simultaneous exposure of myeloma cells to marginally toxic concentrations of L744832 and UCN-01 resulted in a synergistic induction of mitochondrial damage, caspase activation, and apoptosis, associated with activation of p34cdc2 and c-Jun-NH2-kinase and inactivation of extracellular signal-regulated kinase, Akt, GSK-3, p70(S6K), and signal transducers and activators of transcription 3 (STAT3). Enhanced lethality for the combination was also observed in primary CD138+ myeloma cells, but not in their CD138- counterparts. L744832/UCN-01-mediated lethality was not attenuated by conventional resistance mechanisms to cytotoxic drugs (e.g., melphalan or dexamethasone), addition of exogenous interleukin-6 or insulin-like growth factor-I, or the presence of stromal cells. In contrast, enforced activation of STAT3 significantly protected myeloma cells from L744832/UCN-01-induced apoptosis.

Conclusions: Coadministration of the farnesyltransferase inhibitor L744832 promotes UCN-01-induced apoptosis in human multiple myeloma cells through a process that may involve perturbations in various survival signaling pathways, including extracellular signal-regulated kinase, Akt, and STAT3, and through a process capable of circumventing conventional modes of myeloma cell resistance, including growth factor- and stromal cell-related mechanisms. They also raise the possibility that combined treatment with farnesyltransferase inhibitors and UCN-01 could represent a novel therapeutic strategy in multiple myeloma.

Publication types

  • Comparative Study
  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Alkyl and Aryl Transferases / antagonists & inhibitors
  • Antineoplastic Agents / pharmacology
  • Apoptosis / drug effects*
  • Blotting, Western
  • CDC2 Protein Kinase / metabolism
  • Cell Line, Tumor
  • Cytochromes c / metabolism
  • DNA-Binding Proteins
  • Dose-Response Relationship, Drug
  • Drug Synergism
  • Farnesyltranstransferase
  • Glycogen Synthase Kinase 3 / metabolism
  • Humans
  • JNK Mitogen-Activated Protein Kinases / metabolism
  • Methionine / analogs & derivatives*
  • Methionine / pharmacology*
  • Multiple Myeloma / drug therapy
  • Multiple Myeloma / metabolism
  • Multiple Myeloma / pathology
  • Phosphorylation / drug effects
  • Ribosomal Protein S6 Kinases, 70-kDa / metabolism
  • STAT3 Transcription Factor
  • Staurosporine / analogs & derivatives*
  • Staurosporine / pharmacology*
  • Trans-Activators

Substances

  • Antineoplastic Agents
  • DNA-Binding Proteins
  • L 744832
  • STAT3 Transcription Factor
  • STAT3 protein, human
  • Trans-Activators
  • 7-hydroxystaurosporine
  • Cytochromes c
  • Methionine
  • Alkyl and Aryl Transferases
  • Farnesyltranstransferase
  • Ribosomal Protein S6 Kinases, 70-kDa
  • CDC2 Protein Kinase
  • JNK Mitogen-Activated Protein Kinases
  • Glycogen Synthase Kinase 3
  • Staurosporine