Targeting an MMP-9-activated prodrug to multiple myeloma-diseased bone marrow: a proof of principle in the 5T33MM mouse model

Leukemia. 2005 Sep;19(9):1628-33. doi: 10.1038/sj.leu.2403866.

Abstract

Multiple myeloma (MM) is an incurable B-cell cancer characterised by the monoclonal proliferation of tumour cells in the bone marrow (BM). It has been described that matrix metalloproteinases (MMPs) and especially MMP-9 is secreted by MM cells. In this study, we investigated the possibility to exploit MMP-9 activity to activate prodrugs and to target MM cells as a new tumour-specific therapy. Cleavage of the prodrug EV1-FITC by MMP-9 resulted in release of fluorescence which can be used as a measure of prodrug activation. The 5T33MM mouse model was used in this proof-of-principle study. The prodrug was activated in a higher amount by addition to MMP-9-producing 5T33MMvv cells, homogenates from tumour-bearing organs (BM, spleen) and isolated 5T33MM-diseased BM and spleen cells compared to non-MMP-9-producing 5T33MMvt cells and homogenates/cells from non-tumour-bearing organs/mice, as measured by fluorescence release. This fluorescence release could be inhibited by the MMP-2/MMP-9-specific inhibitor, CTT. Activation of the prodrug in the 5T33MM spleen and BM homogenates was confirmed by chromatography. EV1-fluorescein isothiocyanate injection into 5T33MM-diseased animals resulted in a higher fluorescence release by the isolated BM and spleen cells compared to injection into healthy animals. In conclusion, MMP-9 activity can be used to activate prodrugs that target MM.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Biotransformation
  • Bone Marrow Cells / drug effects*
  • Bone Marrow Cells / metabolism
  • Cell Line
  • Disease Models, Animal
  • Dose-Response Relationship, Drug
  • Fluoresceins / chemical synthesis
  • Fluoresceins / metabolism
  • Fluoresceins / therapeutic use*
  • Fluorescence
  • Matrix Metalloproteinase 9 / biosynthesis
  • Matrix Metalloproteinase 9 / metabolism*
  • Mice
  • Mice, Inbred C57BL
  • Molecular Conformation
  • Multiple Myeloma / drug therapy*
  • Multiple Myeloma / metabolism
  • Oligopeptides / chemical synthesis
  • Oligopeptides / metabolism
  • Oligopeptides / therapeutic use*
  • Organ Specificity / drug effects
  • Prodrugs / chemical synthesis
  • Prodrugs / metabolism
  • Prodrugs / therapeutic use*
  • Spleen / cytology
  • Spleen / drug effects
  • Spleen / metabolism

Substances

  • 1-(3-(fluoresceinylthioureidoalanyl-alanyl-alanyl-L-leucyl-glycyl-L-norvalyl-L-prolylamino)propylamino)anthracene-9,10-dione
  • Fluoresceins
  • Oligopeptides
  • Prodrugs
  • Matrix Metalloproteinase 9