[3H]linopirdine binding to rat brain membranes is not relevant for M-channel interaction

Eur J Pharmacol. 2005 Jul 25;518(1):10-7. doi: 10.1016/j.ejphar.2005.06.005.

Abstract

Linopirdine was developed as a cognitive enhancing molecule and demonstrated to specifically block the potassium current generated by the brain specific KCNQ2-KCNQ3 proteins (M-channel). In this study we investigated the relevance of [(3)H]linopirdine binding in rat brain extracts to the interaction with the M-channel proteins. Our results confirm the presence of a high affinity site for [(3)H]linopirdine in rat brain tissues (KD = 10 nM) but we also identified a high affinity binding site for [(3)H]linopirdine in rat liver tissues (KD = 9 nM). Competition experiments showed that [(3)H]linopirdine is displaced by unlabelled linopirdine with comparable affinities from its binding sites on rat brain and rat liver membranes. [(3)H]linopirdine was completely displaced by a set of cytochrome P450 (CYP450) ligands suggesting that [(3)H]linopirdine binding to rat brain and liver membranes is linked to CYP450 interaction. The testing of CYP450 ligands on the M-channel activity, using a Rb(+) efflux assay on cells expressing the KCNQ2-KCNQ3 proteins, demonstrated that [(3)H]linopirdine binding results cannot be correlated to M-channel inhibition. The results obtained in this study demonstrate that [(3)H]linopirdine binding to rat brain and rat liver membranes is representative for CYP450 interaction and not relevant for the binding to the M-channel proteins.

Publication types

  • Comparative Study

MeSH terms

  • Animals
  • Anthracenes / pharmacology
  • Binding, Competitive / drug effects
  • Brain / metabolism*
  • CHO Cells
  • Cell Membrane / metabolism*
  • Chlorides / metabolism
  • Cricetinae
  • Cricetulus
  • Cytochrome P-450 CYP2D6 / metabolism
  • Cytochrome P-450 CYP3A
  • Cytochrome P-450 Enzyme System / metabolism
  • Dose-Response Relationship, Drug
  • Indoles / metabolism*
  • Indoles / pharmacology
  • KCNQ3 Potassium Channel
  • Ketoconazole / pharmacology
  • Kinetics
  • Liver / metabolism
  • Male
  • Miconazole / pharmacology
  • Potassium Channels, Voltage-Gated / antagonists & inhibitors
  • Potassium Channels, Voltage-Gated / genetics
  • Potassium Channels, Voltage-Gated / metabolism*
  • Pyridines / metabolism*
  • Pyridines / pharmacology
  • Pyrilamine / pharmacology
  • Quinidine / pharmacology
  • Radioligand Assay
  • Rats
  • Rats, Sprague-Dawley
  • Rubidium / metabolism
  • Tritium

Substances

  • 10,10-bis(4-pyridinylmethyl)-9(10H)-anthracenone
  • Anthracenes
  • Chlorides
  • Indoles
  • KCNQ3 Potassium Channel
  • Kcnq3 protein, rat
  • Potassium Channels, Voltage-Gated
  • Pyridines
  • Tritium
  • Miconazole
  • Cytochrome P-450 Enzyme System
  • CYP3A protein, human
  • Cytochrome P-450 CYP2D6
  • Cytochrome P-450 CYP3A
  • Pyrilamine
  • linopirdine
  • Quinidine
  • Rubidium
  • rubidium chloride
  • Ketoconazole