Characterisation and biodistribution of two neutral 99mTc(CO)3 complexes with a tridentate ligand

Bioorg Med Chem Lett. 2005 Oct 1;15(19):4192-5. doi: 10.1016/j.bmcl.2005.06.086.

Abstract

N-(2-Mercapto-propyl)-1,2-phenylenediamine (MPPDA) and N-beta-aminoethylglycine (AEG) were labelled with 99mTc(CO)3(+) to form the neutral complexes [99mTc(CO)3(MPPDA)] and [99mTc(CO)3(AEG)]. Both complexes were formed in excellent yields and their identity was confirmed by LC-MS. In mice, none of the new tracer agents showed brain uptake. [(99m)Tc(CO)3(MPPDA)] was trapped mainly in the liver and excreted via the hepatobiliary system, whereas [99mTc(CO)3(AEG)] was excreted rapidly via the kidneys to the urine.

MeSH terms

  • Animals
  • Brain / metabolism
  • Chromatography, High Pressure Liquid
  • Ligands
  • Liver / metabolism
  • Mass Spectrometry
  • Mice
  • Organotechnetium Compounds / chemical synthesis
  • Organotechnetium Compounds / pharmacokinetics*
  • Radiopharmaceuticals / chemical synthesis*
  • Radiopharmaceuticals / pharmacokinetics
  • Tissue Distribution

Substances

  • Ligands
  • Organotechnetium Compounds
  • Radiopharmaceuticals