Molecular basis of listeriolysin O pH dependence

Proc Natl Acad Sci U S A. 2005 Aug 30;102(35):12537-42. doi: 10.1073/pnas.0500558102. Epub 2005 Aug 16.

Abstract

Listeriolysin O (LLO) is a cholesterol-dependent cytolysin that is an essential virulence factor of Listeria monocytogenes. LLO pore-forming activity is pH-dependent; it is active at acidic pH (<6), but not at neutral pH. In contrast to other pH-dependent toxins, we have determined that LLO pore-forming activity is controlled by a rapid and irreversible denaturation of its structure at neutral pH at temperatures >30 degrees C. Rapid denaturation is triggered at neutral pH by the premature unfolding of the domain 3 transmembrane beta-hairpins; structures that normally form the transmembrane beta-barrel. A triad of acidic residues within domain 3 function as the pH sensor and initiate the denaturation of LLO by destabilizing the structure of domain 3. These studies provide a view of a molecular mechanism by which the activity of a bacterial toxin is regulated by pH.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Bacterial Toxins / chemistry*
  • Bacterial Toxins / genetics
  • Bacterial Toxins / toxicity
  • Genes, Bacterial
  • Heat-Shock Proteins / chemistry*
  • Heat-Shock Proteins / genetics
  • Heat-Shock Proteins / toxicity
  • Heat-Shock Proteins / ultrastructure
  • Hemolysin Proteins
  • Hemolysis / drug effects
  • Humans
  • Hydrogen-Ion Concentration
  • In Vitro Techniques
  • Listeria monocytogenes / chemistry
  • Listeria monocytogenes / genetics
  • Listeria monocytogenes / pathogenicity
  • Microscopy, Electron
  • Models, Molecular
  • Multiprotein Complexes
  • Point Mutation
  • Protein Conformation
  • Protein Denaturation
  • Protein Structure, Tertiary
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / genetics
  • Recombinant Proteins / toxicity
  • Recombinant Proteins / ultrastructure
  • Spectrometry, Fluorescence
  • Temperature

Substances

  • Bacterial Toxins
  • Heat-Shock Proteins
  • Hemolysin Proteins
  • Multiprotein Complexes
  • Recombinant Proteins
  • hlyA protein, Listeria monocytogenes