Enzymatic formation of prostamide F2alpha from anandamide involves a newly identified intermediate metabolite, prostamide H2

J Lipid Res. 2005 Dec;46(12):2745-51. doi: 10.1194/jlr.M500374-JLR200. Epub 2005 Sep 8.

Abstract

Prostaglandin F2alpha 1-ethanolamide (prostamide F2alpha) is a potent ocular hypotensive agent in animals and represents a new class of fatty acid amide compounds. Accumulated evidence indicated that anandamide, an endogenous bioactive ligand for cannabinoid receptors, may serve as a common substrate to produce all prostamides, including prostamide F2alpha. After incubation of anandamide with cyclooxygenase 2 (COX-2), the reaction mixture was profiled by HPLC and an intermediate metabolite was discovered and characterized as a cyclic endoperoxide ethanolamide using HPLC-tandem mass spectrometry. Formation of prostamide F2alpha was also demonstrated when the intermediate metabolite was isolated and incubated with prostaglandin F synthase (PGF synthase). These results suggest that the biosynthesis of prostamide F2alpha proceeds in two consecutive steps: oxidation of anandamide to form an endoperoxide intermediate by COX-2, and reduction of the endoperoxide intermediate to form prostamide F2alpha by PGF synthase. This endoperoxide ethanolamide intermediate has been proposed as prostamide H2.

MeSH terms

  • Arachidonic Acids / chemistry
  • Arachidonic Acids / metabolism*
  • Chromatography, High Pressure Liquid
  • Cyclooxygenase 2 / metabolism*
  • Dinoprostone / analogs & derivatives*
  • Dinoprostone / chemistry
  • Dinoprostone / metabolism
  • Endocannabinoids
  • Humans
  • Hydroxyprostaglandin Dehydrogenases / metabolism*
  • Mass Spectrometry
  • Molecular Structure
  • Polyunsaturated Alkamides

Substances

  • Arachidonic Acids
  • Endocannabinoids
  • Polyunsaturated Alkamides
  • prostaglandin F2alpha ethanolamide
  • prostamide H2
  • Hydroxyprostaglandin Dehydrogenases
  • prostaglandin-F synthase
  • Cyclooxygenase 2
  • Dinoprostone
  • anandamide