Concise synthesis of 3,7-dioxa-9-aza-bicyclo[3,3,1]-nonane

J Org Chem. 2006 Jan 6;71(1):413-5. doi: 10.1021/jo051982z.

Abstract

[reaction: see text] The basicity of an amine has a great impact on physicochemical properties and pharmacokinetics. To attenuate the basicity of morpholine, a bicyclic amine was designed and synthesized with the introduction of an additional beta-oxygen. A transannular cyclization and reduction of a bridgehead alpha-chloro amine functionality produces the topographically unusual amine (pKa = 6.7) in good yield.

MeSH terms

  • Alkanes / chemical synthesis*
  • Alkanes / chemistry
  • Aza Compounds / chemical synthesis*
  • Aza Compounds / chemistry
  • Bridged Bicyclo Compounds / chemical synthesis*
  • Bridged Bicyclo Compounds / chemistry
  • Molecular Structure

Substances

  • 3,7-dioxa-9-aza-bicyclo(3,3,1)-nonane
  • Alkanes
  • Aza Compounds
  • Bridged Bicyclo Compounds
  • nonane