Fatty acid amide hydrolase determines anandamide-induced cell death in the liver

J Biol Chem. 2006 Apr 14;281(15):10431-8. doi: 10.1074/jbc.M509706200. Epub 2006 Jan 17.

Abstract

The endocannabinoid anandamide (AEA) induces cell death in many cell types, but determinants of AEA-induced cell death remain unknown. In this study, we investigated the role of the AEA-degrading enzyme fatty acid amide hydrolase (FAAH) in AEA-induced cell death in the liver. Primary hepatocytes expressed high levels of FAAH and were completely resistant to AEA-induced cell death, whereas primary hepatic stellate cells (HSCs) expressed low levels of FAAH and were highly sensitive to AEA-induced cell death. Hepatocytes that were pretreated or with the FAAH inhibitor URB597 isolated from FAAH(-/-) mice displayed increased AEA-induced reactive oxygen species (ROS) formation and were susceptible to AEA-mediated death. Conversely, overexpression of FAAH in HSCs prevented AEA-induced death. Since FAAH inhibition conferred only partial AEA sensitivity in hepatocytes, we analyzed additional factors that might regulate AEA-induced death. Hepatocytes contained significantly higher levels of glutathione (GSH) than HSCs. Glutathione depletion by dl-buthionine-(S,R)-sulfoximine rendered hepatocytes susceptible to AEA-mediated ROS production and cell death, whereas GSH ethyl ester prevented ROS production and cell death in HSCs. FAAH inhibition and GSH depletion had additive effects on AEA-mediated hepatocyte cell death resulting in almost 70% death after 24 h at 50 microm AEA and lowering the threshold for cell death to 500 nm. Following bile duct ligation, FAAH(-/-) mice displayed increased hepatocellular injury, suggesting that FAAH protects hepatocytes from AEA-induced cell death in vivo. In conclusion, FAAH and GSH are determinants of AEA-mediated cell death in the liver.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenoviridae / genetics
  • Amidohydrolases / chemistry*
  • Amidohydrolases / metabolism
  • Animals
  • Apoptosis
  • Arachidonic Acids / pharmacology*
  • Bile Ducts / pathology
  • Blotting, Western
  • Calcium Channel Blockers / pharmacology
  • Cell Death
  • Dose-Response Relationship, Drug
  • Endocannabinoids
  • Fatty Acid Transport Proteins / metabolism
  • Glutathione / metabolism
  • Hepatocytes / metabolism
  • Lipid Metabolism
  • Liver / drug effects*
  • Liver / enzymology*
  • Liver / injuries
  • Liver / metabolism
  • Liver / pathology
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Necrosis
  • Polyunsaturated Alkamides
  • Rats
  • Rats, Sprague-Dawley
  • Reactive Oxygen Species
  • Reverse Transcriptase Polymerase Chain Reaction
  • Time Factors

Substances

  • Arachidonic Acids
  • Calcium Channel Blockers
  • Endocannabinoids
  • Fatty Acid Transport Proteins
  • Polyunsaturated Alkamides
  • Reactive Oxygen Species
  • Amidohydrolases
  • fatty-acid amide hydrolase
  • Glutathione
  • anandamide