Nitroxide SOD-mimics: modes of action

Free Radic Res Commun. 1991:12-13 Pt 1:187-94. doi: 10.3109/10715769109145785.

Abstract

Low molecular weight superoxide dismutase mimics have been shown to afford protection from oxidative damage. Such SOD-mimics can readily permeate cell membrane achieving sufficiently high levels both inside and outside the cell to effectively detoxify intracellular O2-.. Preliminary findings also indicated that metal-based and metal-free SOD-mimics can protect hypoxic cells from H2O2-induced damage. The present study explored the possibility that SOD-mimics such as desferrioxamine-Mn(III) chelate [DF-Mn] or cyclic nitroxide stable free radicals could protect from O2-.-independent damage. Killing of monolayered V79 Chinese hamster cells was induced by H2O2 or by t-butyl hydroperoxide (t-BHP) and assayed clonogenically. Neither catalase nor native SOD protected the cells from t-BHP. In contrast, both DF-Mn and cyclic nitroxides protected suggesting cytotoxic processes independent of O2-. or of O2-.-derived active species. The inhibition of the damage by both metal-free and metal-based SOD mimics is attributable to either SOD-mimic reacting with reduced transition metal to block the Fenton reaction and/or intercepting and detoxifying intracellular organic free radicals.

Publication types

  • Comparative Study

MeSH terms

  • Animals
  • Antioxidants / pharmacology*
  • Catalase / pharmacology
  • Cell Line
  • Cricetinae
  • Cricetulus
  • Cyclic N-Oxides / pharmacology*
  • Cytochrome c Group / metabolism
  • Deferoxamine / pharmacology*
  • Fibroblasts / drug effects
  • Free Radical Scavengers*
  • Free Radicals
  • Hydrogen Peroxide / antagonists & inhibitors
  • Hydrogen Peroxide / pharmacology
  • Lung
  • Models, Chemical
  • Organometallic Compounds / pharmacology
  • Oxidation-Reduction
  • Peroxides / antagonists & inhibitors
  • Peroxides / pharmacology
  • Spin Labels
  • Superoxide Dismutase / pharmacology*
  • Superoxides / metabolism*
  • tert-Butylhydroperoxide

Substances

  • Antioxidants
  • Cyclic N-Oxides
  • Cytochrome c Group
  • Free Radical Scavengers
  • Free Radicals
  • Organometallic Compounds
  • Peroxides
  • Spin Labels
  • Superoxides
  • manganese desferioxamine
  • tert-Butylhydroperoxide
  • Hydrogen Peroxide
  • Catalase
  • Superoxide Dismutase
  • Deferoxamine
  • tempol