The HA2 haemagglutinin domain of the lysine-specific gingipain (Kgp) of Porphyromonas gingivalis promotes micro-oxo bishaem formation from monomeric iron(III) protoporphyrin IX

Microbiology (Reading). 2006 Jun;152(Pt 6):1839-1845. doi: 10.1099/mic.0.28835-0.

Abstract

The lysine- and arginine-specific gingipains (Kgp, and RgpA and RgpB) are the major proteinases produced by the black-pigmented periodontopathogen Porphyromonas gingivalis. They play a role in degrading host proteins, including haemoglobin, from which is formed the mu-oxo bishaem complex of iron(III) protoporphyrin IX, [Fe(III)PPIX]2O, the major haem component of the black pigment. Kgp and RgpA bind haem and haemoglobin via the haemagglutinin-adhesin 2 (HA2) domain, but the role of this domain in the formation of mu-oxo bishaem-containing pigment is not known. UV-visible spectroscopy was used to examine the interaction of iron(III) protoporphyrin IX monomers [Fe(III)PPIX.OH] with recombinant HA2 and purified HRgpA, Kgp and RgpB gingipains. The HA2 domain reacted with Fe(III)PPIX.OH to form mu-oxo bishaem, the presence of which was confirmed by Fourier transform infrared spectroscopy. Both HRgpA and Kgp, but not RgpB, also mediated mu-oxo bishaem formation and aggregation. It is concluded that the Arg- and Lys-gingipains with HA2 haemagglutinin domains may play a crucial role in haem-pigment formation by converting Fe(III)PPIX.OH monomers into [Fe(III)PPIX]2O and promoting their aggregation.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adhesins, Bacterial / chemistry*
  • Adhesins, Bacterial / metabolism*
  • Cysteine Endopeptidases / chemistry*
  • Cysteine Endopeptidases / metabolism*
  • Gingipain Cysteine Endopeptidases
  • Hemagglutinins / chemistry
  • Hemagglutinins / metabolism*
  • Heme / metabolism*
  • Humans
  • Porphyromonas gingivalis / enzymology
  • Porphyromonas gingivalis / metabolism*
  • Protoporphyrins / metabolism*

Substances

  • Adhesins, Bacterial
  • Gingipain Cysteine Endopeptidases
  • Hemagglutinins
  • Protoporphyrins
  • mu-oxo dimeric Fe(III)-protoporphyrin IX
  • Heme
  • protoporphyrin IX
  • Cysteine Endopeptidases