Time-resolved investigation of bright visible wavelength luminescence from sulfur-doped ZnO nanowires and micropowders

Nano Lett. 2006 Jun;6(6):1126-30. doi: 10.1021/nl060204z.

Abstract

Sulfur-doped zinc oxide (ZnO) nanowires grown on gold-coated silicon substrates inside a horizontal tube furnace exhibit remarkably strong visible wavelength emission with a quantum efficiency of 30%, an integrated intensity 1600 times stronger than band edge ultraviolet emission, and a spectral distribution that closely matches the dark-adapted human eye response. By comparatively studying sulfur-doped and undoped ZnO micropowders, we clarify how sulfur doping and nanostructuring affect the visible luminescence and the underlying energy transfer mechanisms.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Equipment Design
  • Equipment Failure Analysis
  • Light
  • Luminescence*
  • Luminescent Measurements / instrumentation*
  • Luminescent Measurements / methods
  • Materials Testing
  • Molecular Conformation
  • Nanostructures / chemistry*
  • Nanostructures / radiation effects*
  • Nanostructures / ultrastructure
  • Particle Size
  • Powders
  • Spectrometry, Fluorescence
  • Sulfur / chemistry*
  • Time Factors
  • Zinc Oxide / chemistry*
  • Zinc Oxide / radiation effects*

Substances

  • Powders
  • Sulfur
  • Zinc Oxide