Solution NMR structure of a human FGF-1 monomer, activated by a hexasaccharide heparin-analogue

FEBS J. 2006 Oct;273(20):4716-27. doi: 10.1111/j.1742-4658.2006.05474.x. Epub 2006 Sep 21.

Abstract

The 3D structure of a complex formed by the acidic fibroblast growth factor (FGF-1) and a specifically designed synthetic heparin hexasaccharide has been determined by NMR spectroscopy. This hexasaccharide can substitute natural heparins in FGF-1 mitogenesis assays, in spite of not inducing any apparent dimerization of the growth factor. The use of this well defined synthetic heparin analogue has allowed us to perform a detailed NMR structural analysis of the heparin-FGF interaction, overcoming the limitations of NMR to deal with the high molecular mass and heterogeneity of the FGF-1 oligomers formed in the presence of natural heparin fragments. Our results confirm that glycosaminoglycans induced FGF-1 dimerization either in a cis or trans disposition with respect to the heparin chain is not an absolute requirement for biological activity.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Binding Sites
  • Carbohydrate Sequence
  • Dimerization
  • Fibroblast Growth Factor 1 / chemistry*
  • Fibroblast Growth Factor 1 / metabolism
  • Heparin / analogs & derivatives*
  • Heparin / chemistry*
  • Heparin / metabolism
  • Humans
  • Magnetic Resonance Spectroscopy
  • Models, Molecular
  • Molecular Sequence Data
  • Multiprotein Complexes / chemistry
  • Oligosaccharides / chemistry*
  • Solutions

Substances

  • Multiprotein Complexes
  • Oligosaccharides
  • Solutions
  • Fibroblast Growth Factor 1
  • Heparin