Structural factors influencing linear M-H-M bonding in bis(dialkylphosphino)methane complexes of nickel

Inorg Chem. 2006 Oct 30;45(22):8853-5. doi: 10.1021/ic0617036.

Abstract

Structural data for four closely related dinuclear nickel hydride complexes have been compared in order to gain insight into the factors governing the Ni-H-Ni geometries. The derivatives [(dippm)2Ni2X2](mu-H) [dippm = 1,2-bis(diisopropylphosphino)methane] were found to contain a linear Ni-H-Ni bridge, whereas the derivatives [(dcpm)2Ni2X2](mu-H) [dcpm = 1,2-bis(dicyclohexylphosphino)methane] were found to contain a bent Ni-H-Ni bridge. The number of internal and interatomic CH-to-halide contacts of the former were much shorter and more numerous than the latter, suggesting an important role of external forces in bridging hydride geometries.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Crystallography, X-Ray
  • Methane / analogs & derivatives*
  • Methane / chemistry
  • Molecular Structure
  • Nickel / chemistry*
  • Organometallic Compounds / chemical synthesis
  • Organometallic Compounds / chemistry*
  • Organophosphorus Compounds / chemical synthesis
  • Organophosphorus Compounds / chemistry*

Substances

  • Organometallic Compounds
  • Organophosphorus Compounds
  • Nickel
  • Methane