Novel pathways associated with quinone-induced stress in breast cancer cells

Drug Metab Rev. 2006;38(4):601-13. doi: 10.1080/03602530600959391.

Abstract

Hormone-dependent breast cancers that overexpress the ligand-binding nuclear transcription factor, estrogen receptor (ER), represent the most common form of breast epithelial malignancy. Exposure of breast epithelial cells to a redox-cycling and arylating quinone induces mitogen-activated protein kinase phosphorylation of the cytoskeletal filament protein, cytokeratin-8, along with thiol arylation of H3 nuclear histones. Exogenous or endogenous quinones can also induce ligand-independent nuclear translocation and phosphorylation of ER; with excess exposure, these quinones can arylate ER zinc fingers, impairing ER DNA-binding and altering ER-inducible gene expression. Immunoaffinity enrichment for low abundance proteins such as ER, coupled with modern mass spectrometry techniques, promises to improve understanding of the protein-modifications produced by endogenous and exogenous quinone exposure and their role in the development or progression of epithelial malignancies such as breast cancer.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Amino Acid Sequence
  • Breast Neoplasms / metabolism*
  • Cell Line, Tumor
  • DNA, Neoplasm / drug effects
  • DNA, Neoplasm / metabolism
  • Female
  • Humans
  • Molecular Sequence Data
  • Oxidative Stress / drug effects*
  • Quinones / pharmacology*
  • Signal Transduction / drug effects

Substances

  • DNA, Neoplasm
  • Quinones