Free radical-mediated pre-hemolytic injury in human red blood cells subjected to lead acetate as evaluated by chemiluminescence

Food Chem Toxicol. 2007 Jun;45(6):945-52. doi: 10.1016/j.fct.2006.12.001. Epub 2006 Dec 12.

Abstract

The mechanisms by which Pb(2+) induces hemolysis are not completely understood. For this reason, the involvement of oxidative stress in the mechanism of Pb(2+)-induced pre-hemolytic lesion was investigated by exposing RBC to Pb(2+) in vitro and then separating the intact non-hemolysed RBC. Oxidative stress was investigated on human RBCs by tert-butyl hydroperoxide-initiated chemiluminescence method (CL). Our results revealed that lead-induced time and concentration-dependent hemolysis and CL time curves showed a very narrow correlation each other. GSH oxidation to GSSG and the stress index also increased significantly. Treatment of lead-exposed RBC with desferrioxamine, an iron-chelating agent or the chain-breaking antioxidant, Trolox, quenched light emission and inhibited hemolysis dramatically. Mannitol and sodium formate, (*)OH scavengers, on the contrary, did not inhibit CL or hemolysis, significantly. These data indicate that lead-induced lipid peroxide formation is mediated by a metal-driven Fenton reaction but do not support the direct involvement of hydroxyl radicals in this process. By contrast, our results revealed a decrease in light emission and decreased hemolysis in the presence of histidine, a singlet oxygen scavenger. Our results suggest that membrane damage and hemolysis of RBC are mediated by Pb(2+) through free radical reactions and that singlet oxygen plays a significant role in this process.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antioxidants / pharmacology
  • Chromans / pharmacology
  • Deferoxamine / pharmacology
  • Erythrocyte Membrane / drug effects*
  • Erythrocytes / drug effects*
  • Erythrocytes / metabolism
  • Formates / pharmacology
  • Free Radicals / metabolism
  • Glutathione / metabolism
  • Hemoglobins / metabolism
  • Hemolysis / drug effects*
  • Hemostatics / pharmacology
  • Histidine / pharmacology
  • Humans
  • Luminescent Measurements / methods
  • Mannitol / pharmacology
  • Organometallic Compounds / toxicity*
  • Oxidative Stress / physiology
  • Siderophores / pharmacology
  • tert-Butylhydroperoxide / metabolism

Substances

  • Antioxidants
  • Chromans
  • Formates
  • Free Radicals
  • Hemoglobins
  • Hemostatics
  • Organometallic Compounds
  • Siderophores
  • formic acid
  • Mannitol
  • Histidine
  • tert-Butylhydroperoxide
  • Glutathione
  • Deferoxamine
  • lead acetate
  • 6-hydroxy-2,5,7,8-tetramethylchroman-2-carboxylic acid