Efficient h/d exchange reactions of alkyl-substituted benzene derivatives by means of the Pd/C-H(2)-D(2)O system

Chemistry. 2007;13(14):4052-63. doi: 10.1002/chem.200601615.

Abstract

A method for efficient and extensive H/D exchange of substituted benzene derivatives which is catalyzed by heterogeneous Pd/C in D(2)O as a deuterium source under hydrogen atmosphere is described. Multi-deuterium incorporation into unactivated linear or branched alkyl chains that bear a carboxyl, hydroxyl, ether, ester, or amide moiety and are connected with a benzene ring was achieved by using the Pd/C-H(2)-D(2)O system. The present method does not require expensive deuterium gas or any special equipment.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzene Derivatives / chemistry*
  • Deuterium Oxide / chemistry*
  • Hydrogen / chemistry*
  • Magnetic Resonance Spectroscopy
  • Palladium / chemistry*

Substances

  • Benzene Derivatives
  • Palladium
  • Hydrogen
  • Deuterium Oxide