Oral bioavailability of curcumin in rat and the herbal analysis from Curcuma longa by LC-MS/MS

J Chromatogr B Analyt Technol Biomed Life Sci. 2007 Jun 15;853(1-2):183-9. doi: 10.1016/j.jchromb.2007.03.010. Epub 2007 Mar 18.

Abstract

This study presents a validated liquid chromatography technique coupled with tandem mass spectrometry (LC-MS/MS) to measure curcumin in rat plasma and provide curcuminoids analysis from the extract of Curcumin longa L. This method was applied to investigate the pharmacokinetics of curcumin in a freely moving rat. The analytes were separated by a reversed phase C18 column (150x4.6 mm I.D., particle size 5 microm) and eluted with acetonitrile-1mM HCOOH mobile phase (70:30, v/v) with a flow rate of 0.8 ml/min in rat plasma and herbal extracts. Multiple reaction monitoring (MRM) was used to monitor the transition of the deprotonated molecule m/z of 367 [M-H]- to the product ion 217 for curcumin, a m/z of 337-217 for demethoxycurcumin and a m/z of 265-224 for honokiol (internal standard) analysis. The limit of detection (LOD) and quantification (LOQ) of curcumin in the rat plasma were 1 and 5 ng/ml, respectively. The method was linear in the range of 5-1000 ng/ml with a coefficient of correlation greater than 0.996 in the rat plasma. After curcumin (500 mg/kg, p.o.) administration, the maximum concentration (Cmax) and the time to reach maximum concentration (Tmax) were 0.06+/-0.01 microg/ml and 41.7+/-5.4 min, respectively. The elimination half-life (t1/2,beta) were 28.1+/-5.6 and 44.5+/-7.5 min for curcumin (500 mg/kg, p.o.) and curcumin (10 mg/kg, i.v.), respectively. The oral bioavailability was about 1%.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Animals
  • Biological Availability
  • Chromatography, Liquid / methods*
  • Curcuma / chemistry*
  • Curcumin / administration & dosage
  • Curcumin / analysis*
  • Curcumin / pharmacokinetics
  • Molecular Structure
  • Plant Extracts / administration & dosage
  • Plant Extracts / analysis
  • Plant Extracts / pharmacokinetics
  • Rats
  • Reproducibility of Results
  • Tandem Mass Spectrometry / methods*

Substances

  • Plant Extracts
  • Curcumin