Micellar electrokinetic chromatography method for the determination of several natural red dyestuff and lake pigments used in art work

J Chromatogr A. 2007 Jun 22;1154(1-2):429-36. doi: 10.1016/j.chroma.2007.03.089. Epub 2007 Mar 30.

Abstract

The identification of organic colorants used in artistic paintings is an important information source for reconstructing the working techniques found in a particular work and for defining a programme for the restoration and conservation of the painting. In this work, sodium dodecyl sulfate (SDS) was used as a surfactant in micellar electrokinetic chromatography (MEKC) for separating a broad range of red organic pigments, based on their colouring matters: madder (colouring matters: alizarin, quinizarin and purpurin), cochineal (colouring matter: carminic acid), red sandalwood (colouring matter: santalin), brazilwood (colouring matter: brazilin), lac dye (colouring matter: laccaic acid) and dragon's blood (colouring matter: dracorhodin). The running electrolyte used was 20 mM borax (pH 9), containing 20 mM SDS and 10% acetonitrile as organic modifier. Separation was carried out by applying a +20 kV voltage at the injection end, 25 degrees C and 214 nm/254 nm as detection wavelengths. All colorants were separated within less than 13 min with a good baseline resolution. The method was applied to the analysis of paint samples obtained from the Diocesan Museum of Holy Art of Bilbao.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Art*
  • Azo Compounds / isolation & purification
  • Benzopyrans / isolation & purification
  • Caesalpinia / chemistry
  • Carmine / analogs & derivatives
  • Carmine / isolation & purification
  • Chromatography, Micellar Electrokinetic Capillary / methods*
  • Color
  • Coloring Agents / analysis*
  • Coloring Agents / isolation & purification
  • Pigments, Biological / analysis
  • Plant Extracts / analysis
  • Plant Extracts / isolation & purification
  • Reproducibility of Results
  • Rubia
  • Santalum / chemistry
  • Sodium Dodecyl Sulfate
  • Uncertainty

Substances

  • Azo Compounds
  • Benzopyrans
  • Coloring Agents
  • Pigments, Biological
  • Plant Extracts
  • madder color
  • lac dye
  • Sodium Dodecyl Sulfate
  • dracorhodin
  • Carmine