Caco-2 cell permeability and stability of two d-glucopyranuronamide conjugates of thyrotropin-releasing hormone

Bioorg Med Chem. 2007 Jul 15;15(14):4946-50. doi: 10.1016/j.bmc.2007.04.042. Epub 2007 Apr 29.

Abstract

Caco-2 cell permeability and stability assays were used as an in vitro model to study the intestinal epithelial transport and stability of two analogues of thyrotropin-releasing hormone (TRH; Pyr-His-Pro-NH2). Peptide 1 (Pyr-His-Pro-D-glucopyranuronamide) was more permeable across the Caco-2 cell monolayer compared with the permeability of the parent TRH peptide (Papp=5.10+/-1.89x10(-6) cm/s c.f. Papp=0.147+/-0.0474x10(-6) cm/s respectively). The permeability of peptide 1 was improved threefold by attaching a 2-aminooctanoic acid moiety to the N-terminus to form peptide 2 (2-aminooctanoic acid-Gln-His-Pro-D-glucopyranuronamide) (Papp=16.3+/-2.47x10(-6) cm/s). The half-life for both peptide 1 and peptide 2 was approximately 20 min in a homogenate of Caco-2 cells compared with the half-life of TRH which is approximately 3 min. It was concluded that the permeability of peptides 1 and 2 was enhanced because of their increased stability, while the higher permeability of peptide 2 compared with peptide 1 may be attributed to its increased lipophilicity which results in enhanced passive diffusion.

MeSH terms

  • Amides / chemistry*
  • Caco-2 Cells
  • Cell Membrane Permeability / drug effects*
  • Glucuronates / chemistry*
  • Humans
  • Molecular Structure
  • Thyrotropin-Releasing Hormone / chemical synthesis
  • Thyrotropin-Releasing Hormone / chemistry*
  • Thyrotropin-Releasing Hormone / pharmacology*

Substances

  • Amides
  • Glucuronates
  • Thyrotropin-Releasing Hormone