Palladium-catalyzed potassium enoxyborate alkylation of enantiopure Hajos-Parrish indenone to construct rearranged steroid ring systems

J Org Chem. 2007 Jun 22;72(13):4837-43. doi: 10.1021/jo070530e. Epub 2007 May 27.

Abstract

Here we report the stereo- and regiospecific C-6 alkylation of a trans-inden-5-one (from optically pure Hajos-Parrish ketone) with allylic electrophiles. Use of this alkylation procedure has led to an improved synthesis of the benz[f]indene ring system and the first enantiospecific total syntheses of the cyclopenta[b]anthracene and cyclopenta[b]phenanthrene ring systems (two synthetic routes).

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Alkylation
  • Anthracenes / chemistry
  • Benzene / chemistry
  • Borates / chemistry*
  • Catalysis
  • Indenes / chemistry*
  • Molecular Structure
  • Palladium / chemistry*
  • Steroids / chemistry*

Substances

  • Anthracenes
  • Borates
  • Indenes
  • Steroids
  • Palladium
  • anthracene
  • Benzene