Cloning and characterization of GDP-perosamine synthetase (Per) from Escherichia coli O157:H7 and synthesis of GDP-perosamine in vitro

Biochem Biophys Res Commun. 2007 Nov 23;363(3):525-30. doi: 10.1016/j.bbrc.2007.08.184. Epub 2007 Sep 10.

Abstract

GDP-perosamine synthetase (Per, E.C. not yet classified) is important to the synthesis of Escherichia coli O157:H7 O-antigen. The mutant in per gene can disrupt the synthesis of O157 O-antigen. In this study, GDP-perosamine synthetase was cloned from E. coli O157:H7 and over-expressed in E. coli BL21 (DE3). The recombinant His-tagged Per fusion protein was a decamer with molecular weight of 431 kDa. The optimal pH value of this recombinant protein was 7.5. The divalent ions had no significant effect on Per-catalyzed reaction. The K(m) and K(cat)/K(m) for GDP-4-keto-6-deoxy-d-mannose were 0.09 mM and 2.1 x 10(5)M(-1)S(-1), and those for l-glutamate were 2mM and 0.52 x 10(5)M(-1)S(-1), respectively. Per was used to synthesize GDP-perosamine from GDP-mannose together with recombinant GDP-mannose dehydratase (GMD, E.C. 4.2.1.47). The purified GDP-perosamine was identified by MS and NMR. In summary, this work provided a feasible approach for the synthesis of GDP-perosamine which can lead to the study of LPS biosynthesis of pathogenic E. coli O157:H7.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Amino Acids / metabolism
  • Binding Sites / genetics
  • Carbohydrate Epimerases / genetics
  • Carbohydrate Epimerases / metabolism*
  • Carbohydrate Sequence
  • Cloning, Molecular
  • Escherichia coli O157 / enzymology*
  • Escherichia coli O157 / genetics
  • Escherichia coli O157 / metabolism
  • Guanosine Diphosphate / metabolism*
  • Hydrogen-Ion Concentration
  • Kinetics
  • Mannose / analogs & derivatives*
  • Mannose / biosynthesis
  • Mannose / chemistry
  • Mannose / metabolism
  • Molecular Sequence Data
  • Molecular Structure
  • Pyridoxal Phosphate / metabolism
  • Recombinant Proteins / metabolism
  • Sequence Homology, Amino Acid
  • Transaminases / genetics
  • Transaminases / metabolism*

Substances

  • Amino Acids
  • Recombinant Proteins
  • Guanosine Diphosphate
  • 4-amino-4,6-dideoxy-D-mannose
  • Pyridoxal Phosphate
  • Transaminases
  • Carbohydrate Epimerases
  • perosamine synthetase
  • Mannose