An enantioselective total synthesis of (+)-aigialospirol

Org Lett. 2007 Nov 8;9(23):4857-9. doi: 10.1021/ol702195w. Epub 2007 Oct 20.

Abstract

A concise and enantioselective total synthesis of (+)-aigialospirol is described here, featuring the first complex natural product synthesis that employs a cyclic ketal-tethered ring-closing metathesis strategy and an unexpected stereoselective epimerization of a benzylic hydroxyl group. The 15-step synthetic sequence illustrates the proof-of-concept that such an approach can be competitive with the classical spiroketal formation in the natural product synthesis.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzofurans / chemical synthesis*
  • Benzofurans / chemistry
  • Crystallography, X-Ray
  • Models, Molecular
  • Molecular Structure
  • Stereoisomerism
  • Zearalenone / analogs & derivatives
  • Zearalenone / chemical synthesis
  • Zearalenone / chemistry

Substances

  • Benzofurans
  • aigialospirol
  • hypothemycin
  • Zearalenone