Synthesis of beta-functionalized porphyrins via palladium-catalyzed carbon-heteroatom bond formations: expedient entry into beta-chiral porphyrins

J Org Chem. 2007 Nov 23;72(24):9060-6. doi: 10.1021/jo701476m. Epub 2007 Oct 24.

Abstract

A procedure was developed for the preparation of beta-monobromo-tetraphenylporphyrin (BrTPP) in a greatly improved yield from the selective bromination of tetraphenylporphyrin (TPP) by NBS. BrTPP was successfully employed as a versatile synthon for convenient synthesis of a wide range of beta-monofunctionalized porphyrins with various heteroatom functionalities via palladium-mediated carbon-heteroatom bond formations. Examples include beta-amino, -amido, -oxo, and -mercaptoporphyrins from reactions with amines, amides, alcohols, and thiols, respectively. Applying the synthetic approach to chiral amides, beta-chiral porphyrins were effectively constructed.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Alcohols / chemistry
  • Amides / chemistry
  • Amines / chemistry
  • Carbon / chemistry*
  • Catalysis
  • Halogenation
  • Models, Chemical
  • Palladium / chemistry*
  • Porphyrins / chemical synthesis*
  • Stereoisomerism
  • Sulfhydryl Compounds / chemistry

Substances

  • Alcohols
  • Amides
  • Amines
  • Porphyrins
  • Sulfhydryl Compounds
  • tetraphenylporphyrin
  • Palladium
  • Carbon