An improved synthesis of cis-4-phenyl-2-propionamidotetralin (4-P-PDOT): a selective MT(2) melatonin receptor antagonist

Org Biomol Chem. 2008 Jan 7;6(1):147-50. doi: 10.1039/b713904g. Epub 2007 Nov 13.

Abstract

A novel, efficient and diastereoselective procedure was developed for the gram-scale synthesis of cis-4-phenyl-2-propionamidotetralin (4-P-PDOT), a selective MT(2) melatonin receptor antagonist. The synthetic strategy involved the conversion of 4-phenyl-2-tetralone to enamide followed by diastereoselective reduction affording cis-4-P-PDOT in good yield. The mechanism of the reduction step was explored by employing deuterated reagents.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Receptor, Melatonin, MT2 / antagonists & inhibitors*
  • Stereoisomerism
  • Tetrahydronaphthalenes / chemical synthesis*
  • Tetrahydronaphthalenes / chemistry
  • Tetrahydronaphthalenes / pharmacology*

Substances

  • 4-phenyl-2-propionamidotetraline
  • Receptor, Melatonin, MT2
  • Tetrahydronaphthalenes